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Rewrite and make corrections in grammar, make APS Reffarance and also check spelling check page numbers and make corrections Fig. 9), which suggests that absorption of this gas takes place in association with a change between a closed and an open structure16. The saturated absorption amount of CO2 was found to be 2.03 mol mol−1 at P/P0 = 0.98 (P ≅ fugacity = 0.99 bar), which corresponds to 1.02 mol per mol of NTf2 ‒. This value is close to those of NTf2 ‒-containing CO2 absorbing ILs at 313 K and 40 bar (fugacity = 34 bar) (under this condition, absorption by NTf2 ‒- containing ILs is ca. 0.5 CO2 mole fraction, corresponding to 1 mol per one mol of NTf2 ‒)17. In order to elucidate the role of fluorinated moieties in governing CO2 absorption, we synthesized the nonfluorinated analog of [Cu(NMes2)2(bpp)2] (2), in which NMes2 ‒ is bis(methylsulfonyl)imide, which has a onedimensional structure that is similar to that of 1 (Supplementary Fig. 6) and measured its absorption properties. As shown in Fig. 3a and Supplementary Fig. 10, CO2 is selectively absorbed to 2 but the threshold pressure in the absorption isotherm (P/P0 = 0.32) is higher than that of 1 (P/P0 = 0.21), indicating that the 

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